1. Mr. Freeze (Batman and Robin, 1997): Menacing, psychotic, bent on Gotham City's destruction...and a master of puns! Here's a couple zingers courtesy of Dr. Victor Fries' frozen-hearted alter ego: "You're not sending me to the cooler." (zing!)
"Ice to see you." (stop...my sides)
"If revenge is a dish best served cold, then put on your Sunday finest. It's time to feast!" (that's not really a pun, but okay)
"Allow me to break the ice. My name is Freeze. Learn it well. For it's the chilling sound of your doom." (um, please stop)
"Let's kick some ice." (that one doesn't even make sense, sir!)
2. Satan (Constantine, 2005): Peter Stormare plays The Prince of Darkness as a drug-addled, homosexual Marlon Brando with attention deficit disorder. The results are, um, confusing?
Two-Face (Batman Forever, 1995): Let's remember Tommy Lee Jones for his wonderful work in films like The Fugitive and No Country for Old Men, not for this shrill, simpering take on one of Batman's greatest enemies. I did like his sexy sidekicks, Sugar and Spice, but for a quality Two-Face, see The Dark Knight.
Galactus (Fantastic Four: Rise of the Silver Surfer, 2007): "Storms a-brewin'. We better head down to the cellar."
Shark (Batman, 1966): Damn sharks! They're always getting in the way when you're trying to save the day. Luckily, back in the 60's, Batman's utility belt included a can of Shark Repellant for just such emergencies.